Charlotte made her debut on a record as far back as 1984 on a track with her father (Serge Gainsbourg) called Lemon Incest then recorded an album titled Charlotte For Ever, but it was her 2006 album 5:55 which was made with the french band Air and other guests that put her on the map musically.
2009 brought the release of her next album IRM which was produced by Beck.
She has a new album out called Stage Whispers which is a companion album to IRM of sorts. It includes songs left over from the IRM sessions (again produced by Beck) and a collection of live tracks. A deluxe edition is to be released late Jan early Feb which will include a bonus dvd disc.