The Louie CK one he posted from 2010 was also great, and the interview with Allie Broosh from Hyperbole and a Half.. aww heck.. I'm just a big fan of WTF..
Lately I've been on the retro gaming podcasts. Back in My Play is pretty good, as is the staple Retronauts. Also Daft Souls is a good UK based podcast, lots of indie games and such, plus most of the people are the same guys who do Shut Up and Sit Down.